Combinatorial structures that compose and decompose give rise to Hopf monoids in Joyal's category of species. The Hadamard product of two Hopf monoids is another Hopf monoid. We prove two main results regarding freeness of Hadamard products. The first one states that if one factor is connected and the other is free as a monoid, their Hadamard product is free (and connected). The second provides an explicit basis for the Hadamard product when both factors are free. The first main result is obtained by showing the existence of a one-parameter deformation of the comonoid structure and appealing to a rigidity result of Loday and Ronco that applies when the parameter is set to zero. To obtain the second result, we introduce an operation on species that is intertwined by the free monoid functor with the Hadamard product. As an application of the first result, we deduce that the Boolean transform of the dimension sequence of a connected Hopf monoid is nonnegative.

Following Radford's proof of Lagrange's theorem for pointed Hopf algebras, we prove Lagrange's theorem for Hopf monoids in the category of connected species. As a corollary, we obtain necessary conditions for a given subspecies $\mathbf k$ of a Hopf monoid $\mathbf h$ to be a Hopf submonoid: the quotient of any one of the generating series of $\mathbf h$ by the corresponding generating series of $\mathbf k$ must have nonnegative coefficients. Other corollaries include a necessary condition for a sequence of nonnegative integers to be the dimension sequence of a Hopf monoid in the form of certain polynomial inequalities, and of a set-theoretic Hopf monoid in the form of certain linear inequalities. The latter express that the binomial transform of the sequence must be nonnegative.